Nature of non-magnetic strongly-correlated state in delta-plutonium

Details Nature of non-magnetic strongly-correlated state in delta-plutonium Nature of non-magnetic strongly-correlated state in delta-plutonium

2005-12-08

arxiv.org/abs/cond-mat/0512185v1

Physics

Condensed Matter

Strongly Correlated Electrons

9 pages, 3 figures

Scientific paper

10.1209/epl/i2005-10548-5

Ab-initio relativistic dynamical mean-field theory is applied to resolve the long-standing controversy between theory and experiment in the "simple" face-centered cubic phase of plutonium called delta-Pu. In agreement with experiment, neither static nor dynamical magnetic moments are predicted. In addition, the quasiparticle density of states reproduces not only the peak close to the Fermi level, which explains the large coefficient of electronic specific heat, but also main 5f features observed in photoelectron spectroscopy.

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