Multiply charged metal cluster anions

Physics – Condensed Matter – Materials Science

Scientific paper

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Latex/Revtex, 4 pages with 4 eps figures integrated in the text. For related papers, see http://www.prism.gatech.edu/~ph274cy

Scientific paper

10.1103/PhysRevLett.86.2996

Formation, stability patterns, and decay channels of silver dianionic and gold trianionic clusters are investigated with Penning-trap experiments and a shell-correction method including shape deformations. The theoretical predictions pertaining to the appearance sizes and electronic shell effects are in remarkable agreement with the experiments. Decay of the multiply anionic clusters occurs predominantly by electron tunneling through a Coulomb barrier, rather than via fission, leading to appearance sizes unrelated to those of multiply cationic clusters.

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