Morphological evolution in a strained-heteroepitaxial solid droplet on a rigid substrate: Dynamical simulations

Details Morphological evolution in a strained-heteroepitaxial solid droplet on a rigid substrate: Dynamical simulations Morphological evolution in a strained-heteroepitaxial solid droplet on a rigid substrate: Dynamical simulations

2010-10-21

arxiv.org/abs/1010.4421v1

JOURNAL OF APPLIED PHYSICS 108, 063527 (2010)

Physics

Condensed Matter

Materials Science

Quantum dots, Instability of surface morphology, Interfaces and surface, Non-equilibrium thermodynamics

Scientific paper

10.1063/1.3483937

A systematic study based on the self-consistent dynamical simulations is presented for the spontaneous evolution of flat solid droplets (bumps), which are driven by the surface drift diffusion induced by the capillary and mismatch stresses, during the development of the Stranski-Krastanow island morphology on a rigid substrate. The physico-mathematical model, which bases on the irreversible thermodynamics treatment of surfaces and interfaces with singularities (Ogurtani, T.O., J. Chem. Phys. 124, 144706, 2006) furnishes us to have auto-control on the otherwise free-motion of the triple junction contour line between the substrate and the droplet without presuming any equilibrium dihedral contract (wetting) angles at the edges. During the development of Stranski-Krastanow islands through the mass accumulation at the central region of the droplet via surface drift-diffusion with and/or without growth, the formation of an extremely thin wetting layer is observed. . This wetting layer has a thickness of a fraction of a nanometer and covers not only the initial computation domain but also its further extension beyond the original boundaries. Above a certain threshold level of the mismatch strain and/or the size (i.e. volume) of the droplets, which depends on the initial physicochemical data and the aspect ratio (i.e., shape) of the original droplet, the formation of the multiple islands separated by the shallow wetting layers is also observed

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