Physics – Condensed Matter – Mesoscale and Nanoscale Physics
Scientific paper
2002-09-04
Physics
Condensed Matter
Mesoscale and Nanoscale Physics
minor corrections (PACS nos, signs in Fig. 2)
Scientific paper
10.1063/1.1543857
In magnetic fields applied parallel to the anisotropy axis, the magnetization of Mn$_{12}$ has been measured in response to a field that is swept back and forth across the resonances corresponding to steps $N=4,5,...9$. The fraction of molecules remaining in the metastable well after each sweep through the resonance is inconsistent with expectations for an ensemble of identical molecules. The data are consistent instead with the presence of a broad distribution of tunnel splittings. A very good fit is obtained for a Gaussian distribution of the second-order anisotropy tunneling parameter $X_E=-\ln(\mid E\mid/2D)$. We show that dipolar shuffling is a negligible effect which cannot explain our data.
Christou George
Hendrickson David N.
Mertes K. M.
Myasoedov Yuri
Rumberger Evan M.
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