Monovalent Ion Condensation at the Electrified Liquid/Liquid Interface

Details Monovalent Ion Condensation at the Electrified Liquid/Liquid Interface Monovalent Ion Condensation at the Electrified Liquid/Liquid Interface

2010-06-23

arxiv.org/abs/1006.4616v1

J. Chem. Phys. 132, 171101 (2010)

Physics

Condensed Matter

Soft Condensed Matter

4 pages, 4 figures

Scientific paper

10.1063/1.3428395

X-ray reflectivity studies demonstrate the condensation of a monovalent ion at the electrified interface between electrolyte solutions of water and 1,2-dichloroethane. Predictions of the ion distributions by standard Poisson-Boltzmann (Gouy-Chapman) theory are inconsistent with these data at higher applied interfacial electric potentials. Calculations from a Poisson-Boltzmann equation that incorporates a non-monotonic ion-specific potential of mean force are in good agreement with the data.

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