Physics
Scientific paper
Jun 2009
adsabs.harvard.edu/cgi-bin/nph-data_query?bibcode=2009mss..confefc03l&link_type=abstract
"International Symposium On Molecular Spectroscopy, 64th Meeting, Held 22-26 June, 2009 at Ohio State University. http://molspec
Physics
Microwave
Scientific paper
The J=2-1 rotational transitions of orthoD_{2}-^{15}N_{2}O and paraD_{2}-^{15}N_{2}O were measured using a microwave-microwave double resonance technique. The experimental setup included a pulsed molecular beam Fourier Transform microwave spectrometer for signal detection and a microwave synthesizer with a K band standard gain horn (frequency range 18 - 26.5 GHz) to generate and transmit the pump radiation. The experimental arrangement was such that the pump radiation propagation was perpendicular to the supersonic molecular expansion. In these experiments, the pump radiation was tuned into resonance with the J_{KaKc}=1_{01}-0_{00} or 1_{11}-0_{00} transition. The resulting population transfer from the rotational ground state facilitated the observation of the J=2-1 transition by significantly enhancing the signal intensity. In addition, a brief update on the solvation studies of nitrous oxide with paraH_{2} molecules will be given.
Endo Yasuki
Jäger Wolfgang
Landry Jen Nicole
Sumiyoshi Yoshihiro
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