Physics – Condensed Matter – Strongly Correlated Electrons
Scientific paper
2009-06-05
Phys. Rev. B 80, 104424 (2009)
Physics
Condensed Matter
Strongly Correlated Electrons
12 pages, 15 figures
Scientific paper
10.1103/PhysRevB.80.104424
The thermodynamic, magnetic, dielectric, and magnetoelectric properties of HoFe$_3$(BO$_3$)$_4$ and Ho$_{0.5}$Nd$_{0.5}$Fe$_3$(BO$_3$)$_4$ are investigated. Both compounds show a second order Ne\'{e}l transition above 30 K and a first order spin reorientation transition below 10 K. HoFe$_3$(BO$_3$)$_4$ develops a spontaneous electrical polarization below the Ne\'{e}l temperature (T$_N$) which is diminished in external magnetic fields. No magnetoelectric effect could be observed in HoFe$_3$(BO$_3$)$_4$. In contrast, the solid solution Ho$_{0.5}$Nd$_{0.5}$Fe$_3$(BO$_3$)$_4$ exhibits both, a spontaneous polarization below T$_N$ and a magnetoelectric effect at higher fields that extends to high temperatures. The superposition of spontaneous polarization, induced by the internal magnetic field in the ordered state, and the magnetoelectric polarizations due to the external field results in a complex behavior of the total polarization measured as a function of temperature and field.
Bezmaternykh Leonard N.
Chaudhury Rajit P.
Chu Cheng-Wei
Lorenz Beat
Sun Yadong
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