Magnetization Step in Spatially Distorted Heisenberg Kagome Antiferromagnets

Physics – Condensed Matter – Strongly Correlated Electrons

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4 pages, 4 figures

Scientific paper

10.1143/JPSJ.79.073708

Motivated by recent experiment for volborthite, a typical spin-1/2 antiferromagnet with kagome lattice structure, we study magnetization process of classical Heisenberg model on a spatially distorted kagome lattice using Monte Carlo (MC) method. We find a distortion-induced magnetization step at low temperatures and low magnetic fields. Magnitude of this step is given by Delta m_z=|1-alpha|/3alpha at zero temperature, where alpha denotes spatial anisotropy in exchange constants. The magnetization step signals a first-order transition at low temperatures, between two phases distinguished by distinct and well developed short-range spin correlations, one characterized by coplanar spin alignment with a \sqrt{3}\times\sqrt{3} period, and the other by a non-coplanar and partially spin flopped structure. We point out the relevance of our results to the unconventional steps observed in volborthite.

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