Physics – Condensed Matter – Strongly Correlated Electrons
Scientific paper
2009-09-28
Phys. Rev. B 80, 134414 (2009)
Physics
Condensed Matter
Strongly Correlated Electrons
17 pages, 10 figures. Accepted for publication in Phys. Rev. B
Scientific paper
10.1103/PhysRevB.80.134414
We describe neutron scattering experiments performed to investigate the magnetic order and dynamics of half-doped La1.5Sr0.5CoO4. This layered perovskite exhibits a near-ideal checkerboard pattern of Co2+/Co3+ charge order at temperatures below ~ 800 K. Magnetic correlations are observed at temperatures below ~ 60 K but static magnetic order only becomes established at 31 K, a temperature at which a kink is observed in the susceptibility. On warming above 31 K we observed a change in the magnetic correlations which we attribute either to a spin canting or to a change in the proportion of inequivalent magnetic domains. The magnetic excitation spectrum is dominated by an intense band extending above a gap of approximately 3 meV up to a maximum energy of 16 meV. A weaker band exists in the energy range 20-30 meV. We show that the excitation spectrum is in excellent quantitative agreement with the predictions of a spin-wave theory generalized to include the full magnetic degrees of freedom of high-spin Co2+ ions in an axially distorted crystal field, coupled by Heisenberg exchange interactions. The magnetic order is found to be stabilized by dominant antiferromagnetic Co2+ -- Co2+ interactions acting in a straight line through Co3+. No evidence is found for magnetic scattering from the Co3+ ions, supporting the view that Co3+ is in the S = 0 state in this material.
Boothroyd Andrew T.
Coldea Radu
Enderle Mechthild
Freeman Paul G.
Frost Carol D.
No associations
LandOfFree
Magnetic order and dynamics of the charge-ordered antiferromagnet La1.5Sr0.5CoO4 does not yet have a rating. At this time, there are no reviews or comments for this scientific paper.
If you have personal experience with Magnetic order and dynamics of the charge-ordered antiferromagnet La1.5Sr0.5CoO4, we encourage you to share that experience with our LandOfFree.com community. Your opinion is very important and Magnetic order and dynamics of the charge-ordered antiferromagnet La1.5Sr0.5CoO4 will most certainly appreciate the feedback.
Profile ID: LFWR-SCP-O-234316