Magnetic Excitation in Artificially Designed Oxygen Molecule Magnet

Physics – Condensed Matter – Strongly Correlated Electrons

Scientific paper

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4 pages, 5 figures, to be published in Journal of Physical Society of Japan

Scientific paper

10.1143/JPSJ.77.083703

We performed inelastic neutron scattering experiment to study magnetic excitation of O$_2$ molecules adsorbed in microporous compound. The dispersionless excitation with characteristic intensity modulation is observed at $\hbar \omega = 7.8$ meV at low temperature. The neutron cross section is explained by spin dimer model with intradimer distance of 3.1 \AA . Anomalous behaviour in the temperature dependence is discussed in the context of enhanced magnetoelasticity in the soft framework of O$_2$ molecule.

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