Macroscopic nucleation phenomena in continuum media with long-range interactions

Details Macroscopic nucleation phenomena in continuum media with long-range interactions Macroscopic nucleation phenomena in continuum media with long-range interactions

2012-01-12

arxiv.org/abs/1201.2495v1

Scientific Reports 1, 162 (2011)

Physics

Condensed Matter

Statistical Mechanics

12 pages, 4 figures. Supplementary information accompanies this paper at http://www.nature.com/scientificreports

Scientific paper

10.1038/srep00162

Nucleation, commonly associated with discontinuous transformations between metastable and stable phases, is crucial in fields as diverse as atmospheric science and nanoscale electronics. Traditionally, it is considered a microscopic process (at most nano-meter), implying the formation of a microscopic nucleus of the stable phase. Here we show for the first time, that considering long-range interactions mediated by elastic distortions, nucleation can be a macroscopic process, with the size of the critical nucleus proportional to the total system size. This provides a new concept of "macroscopic barrier-crossing nucleation". We demonstrate the effect in molecular dynamics simulations of a model spin-crossover system with two molecular states of different sizes, causing elastic distortions.

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