Liquid-gas phase behavior of polydisperse dipolar hard-sphere fluid: Extended TPT-CF

Details Liquid-gas phase behavior of polydisperse dipolar hard-sphere fluid: Extended TPT-CF Liquid-gas phase behavior of polydisperse dipolar hard-sphere fluid: Extended TPT-CF

2009-11-10

arxiv.org/abs/0911.1961v2

Physics

Condensed Matter

Soft Condensed Matter

31 pages, 19 figures

Scientific paper

The liquid-gas phase diagram for polydisperse dipolar hard-sphere fluid with polydispersity in the hard-sphere size and dipolar moment is calculated using extension of the recently proposed thermodynamic perturbation theory for central force (TPT-CF) associating potential. To establish connection with the phase behavior of ferrocolloidal dispersions it is assumed that the dipole moment is proportional to the cube of the hard-sphere diameter. We present the full phase diagram, which includes cloud and shadow curves, binodals and distribution functions of the coexisting daughter phases at different degrees of the system polydispersity.

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