Intrinsic Localized Modes Observed in the High Temperature Vibrational Spectrum of NaI

Physics – Condensed Matter – Strongly Correlated Electrons

Scientific paper

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17 pages, 5 figures Revised version; final version

Scientific paper

10.1103/PhysRevB.79.134304

Inelastic neutron measurements of the high-temperature lattice excitations in NaI show that in thermal equilibrium at 555 K an intrinsic mode, localized in three dimensions, occurs at a single frequency near the center of the spectral phonon gap, polarized along [111]. At higher temperatures the intrinsic localized mode gains intensity. Higher energy inelastic neutron and x-ray scattering measurements on a room-temperature NaI crystal indicate that the creation energy of the ground state of the intrinsic localized mode is 299 meV.

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