Influence of the starting composition on the structural and superconducting properties of MgB2 phase

Physics – Condensed Matter – Superconductivity

Scientific paper

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11 pages, 4 figures

Scientific paper

10.1016/S0921-4534(01)01100-5

We report the preparation of Mg$_{1-x}$B$_{2}$ (0$\le$x$\le$0.5) compounds with the nominal compositions. Single phase MgB$_{2}$ was obtained for x=0 sample. For 0$<$x$\le$0.5, MgB$_{4}$ coexists with "MgB$_{2}$" and the amount of MgB$_{4}$ increases with x. With the increase of x, the lattice parameter ${\it c}$ of "MgB$_{2}$" increases and the lattice parameter ${\it a}$ decreases, correspondingly T$_{c}$ of Mg$_{1-x}$B$_{2}$ decreases. The results were discussed in terms of the presence of Mg vacancies or B interstitials in the MgB$_{2}$ structure. This work is helpful to the understanding of the MgB$_{2}$ films with different T$_{c}$, as well as the Mg site doping effect for MgB$_{2}$.

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