Influence of the lattice geometry on the thermodynamical properties of two-dimensional spin systems

Physics – Condensed Matter – Statistical Mechanics

Scientific paper

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8 pages with 5 Postscript figures, RevTeX, submitted to Phys. Rev. B

Scientific paper

10.1088/0953-8984/10/23/019

Various types of mixed spin two-dimensional Heisenberg networks are investigated by means of Monte Carlo simulations. This study aims at interpreting quantitatively the thermodynamical properties of two-dimensional molecule-based magnets recently synthesized. The proposed model requires that: (i) one of the two magnetic centers has a spin large enough to be treated as a classical spin; (ii) the zero field Hamiltonian is isotropic; (iii) the quantum spins have only classical spins as neighbours. The quantum Hamiltonian is then replaced by a classical one with effective ferromagnetic interactions. The temperature dependence of both the specific heat and magnetic susceptibility are calculated. The effect of the lattice geometry is analysed.

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