Physics – Condensed Matter – Statistical Mechanics
Scientific paper
1997-10-18
Physics
Condensed Matter
Statistical Mechanics
8 pages with 5 Postscript figures, RevTeX, submitted to Phys. Rev. B
Scientific paper
10.1088/0953-8984/10/23/019
Various types of mixed spin two-dimensional Heisenberg networks are investigated by means of Monte Carlo simulations. This study aims at interpreting quantitatively the thermodynamical properties of two-dimensional molecule-based magnets recently synthesized. The proposed model requires that: (i) one of the two magnetic centers has a spin large enough to be treated as a classical spin; (ii) the zero field Hamiltonian is isotropic; (iii) the quantum spins have only classical spins as neighbours. The quantum Hamiltonian is then replaced by a classical one with effective ferromagnetic interactions. The temperature dependence of both the specific heat and magnetic susceptibility are calculated. The effect of the lattice geometry is analysed.
Kahn O.
Leandri J.
Leroyer Yves
Mechkov Serguei
Meurdesoif Y.
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