Physics – Condensed Matter – Strongly Correlated Electrons
Scientific paper
2006-07-12
Phys. Rev. B, 74, 224509, (2006)
Physics
Condensed Matter
Strongly Correlated Electrons
10 pages, 9 figures Phys. Rev. B, 74, 224509, (2006) http://link.aps.org/abstract/PRB/v74/e224509
Scientific paper
We present a detailed Cu K-edge resonant inelastic X-ray scattering (RIXS) study of the Mott insulator La2CuO4 in the 1-7 eV energy transfer range. As initially found for the high-temperature superconductor HgBa2CuO4+d, the spectra exhibit a multiplet of weakly-dispersive electron-hole excitations, which are revealed by utilizing the subtle dependence of the cross section on the incident photon energy. The close similarity between the fine structures for in-plane and out-of-plane polarizations is indicative of the central role played by the 1s core hole in inducing charge excitations within the CuO2 planes. On the other hand, we observe a polarization dependence of the spectral weight, and careful analysis reveals two separate features near 2 eV that may be related to different charge-transfer processes. The polarization dependence indicates that the 4p electrons contribute significantly to the RIXS cross section. Third-order perturbation arguments and a shake-up of valence excitations are then applied to account for the final-energy resonance in the spectra. As an alternative scenario, we discuss fluorescence-like emission processes due to 1s -> 4p transitions into a narrow continuum 4p band.
Casa Diego
Chabot-Couture Guillaume
Gog Th.
Greven Martin
Hancock Jason N.
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