High frequency dielectric and magnetic anomaly at the phase transition in NaV2O5

Physics – Condensed Matter – Strongly Correlated Electrons

Scientific paper

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3 PS-figures, LATEX-text, new experimental data added, typos corrected

Scientific paper

10.1103/PhysRevB.59.14546

We found anomalies in the temperature dependence of the dielectric and the magnetic susceptibiliy of NaV_2O_5 in the microwave and far infrared frequency ranges. The anomalies occur at the phase transition temperature T_c, at which the spin gap opens. The real parts of the dielectric constants epsilon_a and epsilon_c decrease below T_c. The decrease of epsilon_a (except for the narrow region close to T_c) is proportional to the intensity of the x-ray reflection appearing at T_c. The dielectric constant anomaly can be explained by the zigzag charge ordering in the ab-plane appearing below T_c. The anomaly of the microwave magnetic losses is probably related to the coupling between the spin and charge degrees of freedom in vanadium ladders.

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