Heat capacity of the site-diluted spin dimer system Ba3(Mn1-xVx)2O8

Physics – Condensed Matter – Strongly Correlated Electrons

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10.1103/PhysRevB.84.054417

Heat capacity and susceptibility measurements have been performed on the diluted spin dimer compound Ba3(Mn1-xVx)2O8. The parent compound Ba3Mn2O8 is a spin dimer system based on pairs of antiferromagnetically coupled S = 1, 3d2 Mn5+ ions such that the zero field groundstate is a product of singlets. Substitution of non-magnetic S = 0, 3d0 V5+ ions leads to an interacting network of unpaired Mn moments, the low temperature properties of which are explored in the limit of small concentrations, 0

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