Physics – Condensed Matter – Strongly Correlated Electrons
Scientific paper
2007-10-03
Physics
Condensed Matter
Strongly Correlated Electrons
Scientific paper
Inelastic neutron scattering is used to investigate magnetic excitations in the quasi-one-dimensional quantum spin-liquid system Cu2Cl4 D8C4SO2. Contrary to previously conjectured models that relied on bond-alternating nearest neighbor interactions in the spin chains, the dominant interactions are actually next-nearest-neighbor in-chain antiferromagnetic couplings. The appropriate Heisenberg Hamiltonian is equivalent to that of a S = 1/2 4-leg spin-tube with almost perfect one dimensionality and no bond alternation. A partial geometric frustration of rung interactions induces a small incommensurability of short-range spin correlations.
Boehm Manfred
Chung Jae Heon
Garlea Ovidiu V.
Habicht Klaus
Meissner Markus
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