Physics – Condensed Matter
Scientific paper
2000-11-11
Chemical Physics 268, 35-53 (2001)
Physics
Condensed Matter
16 pages, including 1 figure. This version to appear in special issue on dynamics of open quantum systems of Chemical Physics.
Scientific paper
10.1016/S0301-0104(01)00330-5
A central problem in the theory of the dynamics of open quantum systems is the derivation of a rigorous and computationally tractable master equation for the reduced system density matrix. Most generally, the evolution of an open quantum system is described by a completely positive linear map. We show how to derive a completely positive Markovian master equation (the Lindblad equation) from such a map by a coarse graining procedure. We provide a novel and explicit recipe for calculating the coefficients of the master equation, using perturbation theory in the weak-coupling limit. The only parameter external to our theory is the coarse-graining time-scale. We illustrate the method by explicitly deriving the master equation for the spin-boson model. The results are evaluated for the exactly solvable case of pure dephasing, and an excellent agreement is found within the timescale where the Markovian approximation is expected to be valid. The method can be extended in principle to include non-Markovian effects.
Bihary Zsolt
Lidar Daniel A.
Whaley Birgitta K.
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