Free energy for liquids out of equilibrium

Details Free energy for liquids out of equilibrium Free energy for liquids out of equilibrium

2001-06-27

arxiv.org/abs/cond-mat/0106573v1

Physics

Condensed Matter

Soft Condensed Matter

Proceeding for the NATO Advanced Research Workshop "New Kinds of Phase Transitions: Transformations in Disordered Substances"

Scientific paper

Starting for the Stillinger and Weber expression for the free energy of supercooled liquids, we extend the free energy to the case in which two time scales separate and the system is in quasi-equilibrium. The concept of an effective temperature, different from the kinetic temperature, is naturally introduced. An example of hypotetical quasi-equilibrium phase diagram is presented for the case of SPC/E water.

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