Fast recognition of single molecules based on single event photon statistics

Physics – Quantum Physics

Scientific paper

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13 pages, 4figures

Scientific paper

10.1103/PhysRevA.76.063820

Mandel Q-parameter, which is determined from single event photon statistics, provides an alternative to differentiate single-molecule with fluorescence detection. In this work, by using the Q-parameter of the sample fluorescence compared to that of an ideal double-molecule system with the same average photon number, we present a novel and fast approach for identifying single molecules based on single event photon statistics analyses, compared with commonly used two-time correlation measurements. The error estimates for critical values of photon statistics are also presented for single-molecule determination.

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