Electronic structure of CdTe nanocrystals: A tight-binding study

Physics – Condensed Matter – Mesoscale and Nanoscale Physics

Scientific paper

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9 pages, 5 eps figures, to be published in Solid State Comm

Scientific paper

10.1016/S0038-1098(99)00064-2

We present a symmetry-based calculation of the electronic structure of a compound semiconductor quantum dot (QD) in the sp^3s* tight-binding model including the spin-orbit interaction. The Hamiltonian matrix is diagonalized exactly for CdTe QD sizes up to 60 {\AA}. The surface dangling bonds are passivated by hydrogen through a careful analysis of the density of states and wave functions. The calculated size dependence of the energy gap shows a reasonable agreement with the available experimental data. Our symmetry analysis indicates that, in contrast with a reported prediction of the three-band effective-mass model, the fundamental interband transition remains dipole-allowed in CdTe nanocrystals.

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