Electronic structure of C60 / graphite

Details Electronic structure of C60 / graphite Electronic structure of C60 / graphite

2001-08-07

arxiv.org/abs/cond-mat/0108111v1

Physics

Condensed Matter

Strongly Correlated Electrons

Proc. of the XV. Int. Winterschool on Electronic Properties of Novel Materials, Kirchberg/Tirol, Austria, 2001

Scientific paper

We report temperature-dependent photoelectron spectra for a monolayer of C_60 adsorbed on HOPG, as well as C 1s x-ray absorption. This extends a previous report which showed the close similarity between the spectrum of the HOMO for the two-dimensional overlayer and that of C_60 in the gas phase. The present work shows that intermolecular and molecule-substrate vibrations contribute strongly to the spectral lineshape at room temperature. Thus, vibrational effects are shown to be crucial for the proper understanding of photoelectron spectra, and thus the charge transport properties, for C_60 in contact with graphite and graphite-like materials.

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