Physics – Condensed Matter – Strongly Correlated Electrons
Scientific paper
2008-04-25
Acta Physica 18 (2008) 1
Physics
Condensed Matter
Strongly Correlated Electrons
4 pages, 2 figures embedded
Scientific paper
Magnetic properties of stechiometric Cs2AgF4 have been calculated within a very strong correlation limit taking into account a low-symmetry crystal field and the intra-atomic spin-orbit coupling of the Ag2+ ion. We consistently explain the insulating ground state and the magnetic state revealing the spin gap of 2.6 meV below Tc of 14.9 K. A d-d excitation of 2.0-2.3 eV related to the t2g-eg promotion energy (=10Dq) is a reason for the lilac colour of Cs2AgF4. Our approach can be experimentally verified by the measurement of the g factor (gz =2.12 and gy =2.52) and the absorption energy at 2.0-2.3 eV.
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