Electronic excitations of a single molecule contacted in a three-terminal configuration

Details Electronic excitations of a single molecule contacted in a three-terminal configuration Electronic excitations of a single molecule contacted in a three-terminal configuration

2007-11-16

arxiv.org/abs/0711.2592v1

Nano lett. 2007, 7, 3336

Physics

Condensed Matter

Mesoscale and Nanoscale Physics

Supporting information avalaible at http://pubs.acs.org

Scientific paper

10.1021/nl0715802

Low-temperature three-terminal transport measurements through a thiol end-capped Pi -conjugated molecule have been carried out. Electronic excitations, including zero and finite-bias Kondo-effects have been observed and studied as a function of magnetic field. Using a simplified two-orbital model we have accounted for the spin and the electronic configuration of the first four charge states of the molecule. The charge-dependent couplings to gate, source and drain electrodes suggest a scenario in which charges and spins are localized at the ends of the molecule, close to the electrodes.

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