Electromagnetic response of broken-symmetry nano-scale clusters

Physics – Condensed Matter – Strongly Correlated Electrons

Scientific paper

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Scientific paper

10.1103/PhysRevLett.97.036806

A microscopic, non-local response theory is developed to model the interaction of electromagnetic radiation with inhomogeneous nano-scale clusters. The breakdown of classical continuum-field Mie theory is demonstrated at a critical coarse-graining threshold, below which macroscopic plasmon resonances are replaced by molecular excitations with suppressed spectral intensity.

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