Physics – Condensed Matter – Strongly Correlated Electrons
Scientific paper
2007-03-16
Physical Review Letters 99, 057204 (2007)
Physics
Condensed Matter
Strongly Correlated Electrons
4 pages, 4 figures now identical with finally published version
Scientific paper
10.1103/PhysRevLett.99.057204
By means of thermal expansion and specific heat measurements on the high-pressure phase of (VO)$_2$P$_2$O$_7$, the effects of two energy scales of the weakly dimerized antiferromagnetic $S$ = 1/2 Heisenberg chain are explored. The low energy scale, given by the spin gap $\Delta$, is found to manifest itself in a pronounced thermal expansion anomaly. A quantitative analysis, employing T-DMRG calculations, shows that this feature originates from changes in the magnetic entropy with respect to $\Delta$, $\partial S^{m}/ \partial \Delta$. This term, inaccessible by specific heat, is visible only in the weak-dimerization limit where it reflects peculiarities of the excitation spectrum and its sensitivity to variations in $\Delta$.
Anton M.
Assmus Wolf
Brühl Andreas
Glocke S.
Gross Christian
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