Physics – Condensed Matter – Strongly Correlated Electrons
Scientific paper
2008-11-04
PHYSICAL REVIEW B 77, 235118 (2008)
Physics
Condensed Matter
Strongly Correlated Electrons
Scientific paper
10.1103/PhysRevB.77.235118
We investigate the low temperature magnetic field dependence of the resistivity in the thermoelectric misfit cobalt oxide [Bi1.7Ca2O4]0.59CoO2 from 60 K down to 3 K. The scaling of the negative magnetoresistance demonstrates a spin dependent transport mechanism due to a strong Hund's coupling. The inferred microscopic description implies dual electronic states which explain the coexistence between localized and itinerant electrons both contributing to the thermopower. By shedding a new light on the electronic states which lead to a high thermopower, this result likely provides a new potential way to optimize the thermoelectric properties.
Fresard Raymond
Hebert Sylvie
Limelette Patrice
Muguerra Herve
Simon Charles
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