Direct Evidence for the Localized Single-Triplet Excitations and the Dispersive Multi-Triplets Excitations in SrCu2(BO3)2

Physics – Condensed Matter – Strongly Correlated Electrons

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12 pages, with 4 figures, to appear in Phys. Rev. Lett

Scientific paper

10.1103/PhysRevLett.84.5876

We performed inelastic neutron scattering on the 2D Shastry-Sutherland system SrCu2(11BO3)2 with an exact dimer ground state. Three energy levels at around 3, 5 and 9 meV were observed at 1.7 K. The lowest excitation at 3.0 meV is almost dispersionless with a bandwidth of 0.2 meV at most, showing a significant constraint on a single-triplet hopping owing to the orthogonality of the neighboring dimers. In contrast, the correlated two-triplets excitations at 5 meV exhibit a more dispersive behavior.

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