Physics – Condensed Matter – Statistical Mechanics
Scientific paper
1999-12-13
Eur. Phys. J. B 14, 139-144 (2000)
Physics
Condensed Matter
Statistical Mechanics
21 pages, no figure, to be published in EPJ B
Scientific paper
10.1007/s100510050114
We study a single, motionless three-dimensional droplet growing by adsorption of diffusing monomers on a 2D substrate. The diffusing monomers are adsorbed at the aggregate perimeter of the droplet with different boundary conditions. Models with both an adsorption boundary condition and a radiation boundary condition, as well as a phenomenological model, are considered and solved in a quasistatic approximation. The latter two models allow particle detachment. In the short time limit, the droplet radius grows as a power of the time with exponents of 1/4, 1/2 and 3/4 for the models with adsorption, radiation and phenomenological boundary conditions, respectively. In the long time limit a universal growth rate as $[t/\ln(t)]^{1/3}$ is observed for the radius of the droplet for all models independent of the boundary conditions. This asymptotic behaviour was obtained by Krapivsky \cite{krapquasi} where a similarity variable approach was used to treat the growth of a droplet with an adsorption boundary condition based on a quasistatic approximation. Another boundary condition with a constant flux of monomers at the aggregate perimeter is also examined. The results exhibit a power law growth rate with an exponent of 1/3 for all times.
Rodgers Geoff J.
Tavassoli Z.
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