Physics – Condensed Matter – Superconductivity
Scientific paper
2001-10-12
Physics
Condensed Matter
Superconductivity
To be published in PRB
Scientific paper
10.1103/PhysRevB.64.184428
The title quasi-1D copper oxides (0=< x =<0.4) were investigated by neutron diffraction and magnetic susceptibility studies. Polyhedral CuO4 units in the compounds were found to comprise linear-chains at inter-chain distance of approximately 10 A. The parent chain compound (x = 0), however, shows less anisotropic magnetic behavior above 2 K, although it is of substantially antiferromagnetic (mu_{eff}= 1.85 mu_{B} and Theta_{W} = -46.4 K) spin-chain system. A magnetic cusp gradually appears at about 100 K in T vs chi with the Bi substitution. The cusp (x = 0.4) is fairly characterized by and therefore suggests the spin gap nature at Delta/k_{B} ~ 80 K. The chain compounds hold electrically insulating in the composition range.
Huang Qingzhen
Takayama-Muromachi Eiji
Yamaura Kazunari
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