Physics – Condensed Matter – Mesoscale and Nanoscale Physics
Scientific paper
1999-03-10
Phys. Rev. B 59, 6309(1999)
Physics
Condensed Matter
Mesoscale and Nanoscale Physics
10 pages, 3 figures
Scientific paper
10.1103/PhysRevB.59.6309
The crossover from thermal hopping to quantum tunneling is studied. We show that the decay rate $\Gamma$ with dissipation can accurately be determined near the crossover temperature. Besides considering the Wentzel-Kramers-Brillouin (WKB) exponent, we also calculate contribution of the fluctuation modes around the saddle point and give an extended account of a previous study of crossover region. We deal with two dangerous fluctuation modes whose contribution can't be calculated by the steepest descent method and show that higher order couplings between the two dangerous modes need to be taken into considerations. At last the crossover from thermal hopping to quantum tunneling in the molecular magnet Mn_{12}Ac is studied.
Kou Su-Peng
Liang Jing-Qiu
Pu Fu-Cho
Wang Xiang-Bin
Zhang Y.-B.
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