Correlated Electron Transport

Details Correlated Electron Transport Correlated Electron Transport

2003-12-19

arxiv.org/abs/cond-mat/0312522v1

Physics

Condensed Matter

4 pages with 3 figures

Scientific paper

Theoretical and experimental values to date for the resistances of single molecules commonly disagree by orders of magnitude. By reformulating the transport problem using boundary conditions suitable for correlated many-electron systems, we approach electron transport across molecules from a new standpoint. Application of our correlated formalism to benzene-dithiol gives current-voltage characteristics close to experimental observations. The method can solve the open system quantum many-body problem accurately, treats spin exactly and is valid beyond the linear response regime.

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