Physics – Condensed Matter – Mesoscale and Nanoscale Physics
Scientific paper
2012-01-10
Physics
Condensed Matter
Mesoscale and Nanoscale Physics
8 pages, 6 figures, submitted to PRL
Scientific paper
We demonstrate strong coupling between molecular excited states and surface plasmon modes of a slit array in a thin metal film. The coupling manifests itself as an anti-crossing behavior of the two newly formed polaritons. As the coupling strength grows, a new mode emerges, which is attributed to long range molecular interactions mediated by the plasmonic field. The new, molecular-like mode repels the polariton states, and leads to an opening of energy gaps both below and above the asymptotic free molecule energy.
Gordon Robert J.
Prior Yehiam
Salomon Adi
Seideman Tamar
Sukharev Maxim
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