Clathrate hydrate of carbon dioxide above 0.2 GPa: new experimental results and theoretical developments

Details Clathrate hydrate of carbon dioxide above 0.2 GPa: new experimental results and theoretical developments Clathrate hydrate of carbon dioxide above 0.2 GPa: new experimental results and theoretical developments

Oct 2011

adsabs.harvard.edu/cgi-bin/nph-data_query?bibcode=2011epsc.conf.1228b&link_type=abstract

EPSC-DPS Joint Meeting 2011, held 2-7 October 2011 in Nantes, France. http://meetings.copernicus.org/epsc-dps2011, p.1228

Physics

Scientific paper

New diamond anvil cell experiments were carried out to explore the stability of the CO2 sI clathrate hydrate. Our results support the existence of a "highpressure" structure above 0.6~0.8 GPa and provide the first Raman analysis for this new phase. Ongoing experiments in the H2O-CO2 system are performed to constrain the carbon dioxide solubility in water above 0.2 GPa. These results will help to improve the thermodynamic model of aqueous solutions developed in Nantes.

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