Physics – Condensed Matter – Mesoscale and Nanoscale Physics
Scientific paper
2007-07-13
Physics
Condensed Matter
Mesoscale and Nanoscale Physics
15 pages, 3 figures
Scientific paper
We propose a novel mechanism for photogeneration of multiexcitons by single photons (carrier multiplication) in semiconductor nanocrystals. In this mechanism, the Coulomb interaction between two valence-band electrons involving their transfer to the conduction band creates a virtual biexciton from vacuum that is then converted into a real biexciton by photon absorption on an intraband optical transition. This mechanism is inactive in bulk semiconductors as momentum conservation suppresses intraband absorption. However, it becomes highly efficient in zero-dimensional nanocrystals and can provide a significant contribution to carrier multiplication in these materials.
Klimov Victor I.
Rupasov Valery I.
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