Berry-Phase induced Heat Pumping and its Impact on the Fluctuation Theorem

Physics – Condensed Matter – Mesoscale and Nanoscale Physics

Scientific paper

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8 pages, 4 figures. Accepted by Physcial Review Letters. Supplementary file is included, which presents a detailed derivation

Scientific paper

10.1103/PhysRevLett.104.170601

Applying adiabatic, cyclic two parameter modulations we investigate quantum heat transfer across an anharmonic molecular junction contacted with two heat baths. We demonstrate that the pumped heat typically exhibits a Berry phase effect in providing an additional geometric contribution to heat flux. Remarkably, a robust fractional quantized geometric phonon response is identified as well. The presence of this geometric phase contribution in turn causes a breakdown of the fluctuation theorem of the Gallavotti-Cohen type for quantum heat transfer. This can be restored only if (i) the geometric phase contribution vanishes and if (ii) the cyclic protocol preserves the detailed balance symmetry.

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