Physics – Chemical Physics
Scientific paper
2009-06-05
Phys.Rev.Lett. 103, 103002 (2009)
Physics
Chemical Physics
Scientific paper
10.1103/PhysRevLett.103.103002
Laser pulses with stable electric field waveforms establish the opportunity to achieve coherent control on attosecond timescales. We present experimental and theoretical results on the steering of electronic motion in a multi-electron system. A very high degree of light-waveform control over the directional emission of C+ and O+ fragments from the dissociative ionization of CO was observed. Ab initio based model calculations reveal contributions to the control related to the ionization and laser-induced population transfer between excited electronic states of CO+ during dissociation.
de Vivie-Riedle Regina
den Hoff von P.
Herrwerth O.
Kling Matthias F.
Vrakking M. J. J.
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