Physics – Condensed Matter – Strongly Correlated Electrons
Scientific paper
2007-08-10
Phys. Rev. B 76, 245119 (2007)
Physics
Condensed Matter
Strongly Correlated Electrons
6 pages, 5 figures
Scientific paper
10.1103/PhysRevB.76.245119
We have performed angle-dependent near-edge x-ray absorption fine structure measurements in the Auger electron yield mode on the correlated quasi-one-dimensional organic conductor TTF-TCNQ in order to determine the orientation of the molecules in the topmost surface layer. We find that the tilt angles of the molecules with respect to the one-dimensional axis are essentially the same as in the bulk. Thus we can rule out surface relaxation as the origin of the renormalized band widths which were inferred from the analysis of photoemission data within the one-dimensional Hubbard model. Thereby recent theoretical results are corroborated which invoke long-range Coulomb repulsion as alternative explanation to understand the spectral dispersions of TTF-TCNQ quantitatively within an extended Hubbard model.
Blaha Peter
Claessen Ralph
Gavrila Gianina
Glawion Sebastian
Hoinkis Markus
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