Anomaly in the dielectric response at the charge orbital ordering transition of crystalline Pr0.67Ca0.33MnO3

Details Anomaly in the dielectric response at the charge orbital ordering transition of crystalline Pr0.67Ca0.33MnO3 Anomaly in the dielectric response at the charge orbital ordering transition of crystalline Pr0.67Ca0.33MnO3

2003-04-11

arxiv.org/abs/cond-mat/0304281v2

Physics

Condensed Matter

Strongly Correlated Electrons

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Scientific paper

10.1103/PhysRevB.69.174433

The complex impedance of a Pr0.67Ca0.33MnO3 crystal has been measured. The frequency dependence is studied for a wide range of temperatures (50K-403K) and is found to be characteristic of relaxation process with a single Debye time relaxation constant, which is interpreted as a dielectric constant of the material. A strong peak is observed in this dielectric constant (up to two millions) at the charge ordering transition suggesting an interpretation in terms of ordering of electric dipoles at TCO or in term of phase separation. Comparison with Pr0.63Ca0.37MnO3 - in which the phase separation is much smaller and the peak in the dielectric constant is absent - suggests an interpretation in term of phase separation between insulating and metallic states.

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