Physics – Condensed Matter – Strongly Correlated Electrons
Scientific paper
2011-02-17
Phys. Rev. B 83, 245127 (2011)
Physics
Condensed Matter
Strongly Correlated Electrons
17 pages, 3 figures
Scientific paper
Polarized Raman-scattering spectra of non-superconducting, single-crystalline FeTe are investigated as function of temperature. We have found a relation between the magnitude of ordered magnetic moments and the linewidth of A1g phonons at low temperatures. This relation is attributed to the intermediate spin state (S=1) and the orbital degeneracy of the Fe ions. Spin-phonon coupling constants have been estimated based on microscopic modeling using density-functional theory and analysis of the local spin density. Our observations show the importance of orbital degrees of freedom for the Fe-based superconductors with large ordered magnetic moments, while small magnetic moment of Fe ions in some iron pnictides reflects the low spin state of Fe ions in those systems.
Afanasiev O.
Deisenhofer Joachim
Gnatchenko S.
Gnezdilov Vladimir
Gusev Alexander A.
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