Anomalous magnetic phase in an undistorted pyrochlore oxide Cd2Os2O7 induced by geometrical frustration

Details Anomalous magnetic phase in an undistorted pyrochlore oxide Cd2Os2O7 induced by geometrical frustration Anomalous magnetic phase in an undistorted pyrochlore oxide Cd2Os2O7 induced by geometrical frustration

2007-02-07

arxiv.org/abs/cond-mat/0702164v2

J. Phys. Soc. Jpn. 76, 063703 (2007).

Physics

Condensed Matter

Strongly Correlated Electrons

5 pages, 4 figures

Scientific paper

10.1143/JPSJ.76.063703

We report on the muon spin rotation/relaxation study of a pyrochlore oxide, Cd2Os2O7, which exhibits a metal-insulator (MI) transition at T_{MI}~225 K without structural phase transition. It reveals strong spin fluctuation (>10^8/s) below the MI transition, suggesting a predominant role of geometrical spin frustration amongst Os^{5+} ions. Meanwhile, upon further cooling, a static spin density wave discontinuously develops below T_{SDW}~150 K. These observations strongly suggest the occurrence of an anomalous magnetic transition and associated change in the local spin dynamics in undistorted pyrochlore antiferromagnet.

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