Physics – Condensed Matter – Materials Science
Scientific paper
2010-01-16
Nano Lett. 9, 4234-4239 (2009)
Physics
Condensed Matter
Materials Science
Scientific paper
10.1021/nl902448v
Angle-resolved photoemission spectroscopy (ARPES) is a powerful experimental technique for directly probing electron dynamics in solids. The energy vs. momentum dispersion relations and the associated spectral broadenings measured by ARPES provide a wealth of information on quantum many-body interaction effects. In particular, ARPES allows studies of the Coulomb interaction among electrons (electron-electron interactions) and the interaction between electrons and lattice vibrations (electron-phonon interactions). Here, we report ab initio simulations of the ARPES spectra of graphene including both electron-electron and electron-phonon interactions on the same footing. Our calculations reproduce some of the key experimental observations related to many-body effects, including the indication of a mismatch between the upper and lower halves of the Dirac cone.
Cohen Marvin L.
Giustino Feliciano
Louie Steven G.
Park Cheol-Hwan
Spataru Catalin D.
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