Adsorbate Interactions of CO Chemisorbed on Pt(111)

Details Adsorbate Interactions of CO Chemisorbed on Pt(111) Adsorbate Interactions of CO Chemisorbed on Pt(111)

1997-12-02

arxiv.org/abs/cond-mat/9712026v1

Physics

Condensed Matter

LaTeX2e, Elsevier Preprint, 11 pages, 2 eps figures, Submitted to Surface Science Letters

Scientific paper

10.1016/S0039-6028(98)00074-0

We show that the observed repulsive interaction between CO molecules on the Pt(111) surface can be explained by the coupling of the Pt--CO separation with Pt-Pt coordinates in the substrate. The observed long range of the interaction and the non-monotonic distance dependence are reproduced. The magnitude of the multiphonon decay of the Pt--CO vibration calculated in this model is also in agreement with experiment.

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