Adlayer core-level shifts of admetal monolayers on transition metal substrates and their relation to the surface chemical reactivity

Physics – Condensed Matter – Materials Science

Scientific paper

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RevTeX, 7 pages, 2 figures

Scientific paper

10.1103/PhysRevB.53.10344

Using density-functional-theory we study the electronic and structural properties of a monolayer of Cu on the fcc (100) and (111) surfaces of the late 4d transition metals, as well as a monolayer of Pd on Mo bcc(110). We calculate the ground states of these systems, as well as the difference of the ionization energies of an adlayer core electron and a core electron of the clean surface of the adlayer metal. The theoretical results are compared to available experimental data and discussed in a simple physical picture; it is shown why and how adlayer core-level binding energy shifts can be used to deduce information on the adlayer's chemical reactivity.

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