A slow process in confined polymer melts: layer exchange dynamics at a polymer solid interface

Details A slow process in confined polymer melts: layer exchange dynamics at a polymer solid interface A slow process in confined polymer melts: layer exchange dynamics at a polymer solid interface

2010-09-16

arxiv.org/abs/1009.3211v1

Physics

Condensed Matter

Soft Condensed Matter

Scientific paper

Employing Molecular Dynamics simulations of a chemically realistic model of
1,4-polybutadiene between graphite walls we show that the mass exchange between
layers close to the walls is a slow process already in the melt state. For the
glass transition of confined polymers this process competes with the slowing
down due to packing effects and intramolecular rotation barriers.

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