A correlation between the equilibrium and transport properties of intercalation systems

Details A correlation between the equilibrium and transport properties of intercalation systems A correlation between the equilibrium and transport properties of intercalation systems

2003-06-23

arxiv.org/abs/cond-mat/0306559v1

Physics

Condensed Matter

Statistical Mechanics

7 pages, 5 figures

Scientific paper

Employing the lattice gas model, combined with the linear elasticity theory, a correlation between the equilibrium and transport properties of intercalated species is investigated. It is shown that the major features of the intercalation isotherms and the concentration dependence of the chemical diffusion coefficient can be well understood in terms of the change of the host volume in the course of intercalation. Theoretical predictions are compared to the experimental observations on PdH_x, Li_xWO_3 and Li-graphite systems.

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