17O NMR study of q=0 spin excitations in a nearly ideal S=1/2 1D Heisenberg antiferromagnet, Sr2CuO3, up to 800 K

Physics – Condensed Matter – Strongly Correlated Electrons

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Submitted to Phys. Rev. Lett. 4 pages, 4 figures

Scientific paper

10.1103/PhysRevLett.87.247202

We used 17O NMR to probe the uniform (wavevector q=0) electron spin excitations up to 800 K in Sr2CuO3 and separate the q=0 from the q=\pm\pi/a staggered components. Our results support the logarithmic decrease of the uniform spin susceptibility below T ~ 0.015J, where J=2200 K. From measurement of the dynamical spin susceptibility for q=0 by the spin-lattice relaxation rate 1/T_{1}, we demonstrate that the q=0 mode of spin transport is ballistic at the T=0 limit, but has a diffusion-like contribution at finite temperatures even for T << J.

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