Physics – Condensed Matter
Scientific paper
1993-07-06
J. Luminescence 60&61 (1994) 380-382
Physics
Condensed Matter
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Scientific paper
10.1016/0022-2313(94)90170-8
The third-order nonlinear optical susceptiblity chi(3) of a C60 molecule is calculated by using a free-electron model as well as by taking Coulomb interactions into account. The free-electron model yields chi(3) magnitudes which are in agreement with experiment. Althugh Coulomb interactions reduce chi(3) by one order of magnitude, local-field corrections can be invoked to recover the agreement.
Abe Shuji
Harigaya Kikuo
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